Super-high-frequency shielding properties of excimer-laser-synthesized- single-wall-carbon-nanotubes/polyurethane nanocomposite films

Brahim Aissa, L. L. Laberge, M. A. Habib, T. A. Denidni, D. Therriault, M. A. El Khakani

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Abstract

Electromagnetic shielding attenuation (ESA) properties of carbon nanotubes/polymer nanocomposite films, in the super high frequency (SHF) X-band (7-12 GHz) domain are studied. The nanocomposite films consisted of thermoset polyurethane (PU) resin blended with single-walled carbon nanotubes (SWCNTs) mats, and deposited on fused quartz substrates. Two different approaches were used to achieve the nanocomposite films, namely (i) through the on-substrate "all-laser" growth approach of SWCNTs directly onto substrate, followed by their infiltration by the PU resin, and (ii) by appropriately dispersing the chemically-purified SWCNTs (in the soot form) into the PU matrix and their subsequent deposition onto quartz substrates by means of a solvent casting process. Characterizations of the ESA properties of the developed nanocomposite films show that they exhibit systematically a deep shielding band, centered at around 9.5 GHz, with an attenuation as high as |- 30| dB, recorded for SWCNT loads of 2.5 wt. % and above. A direct correlation is established between the electrical conductivity of the nanocomposite films and their electromagnetic shielding capacity. The SWCNTs/PU nanocomposites developed here are highly promising shielding materials as SHF notch filters, as their ESA capacity largely exceeds the target value of |- 20| dB generally requested for commercial applications.

Original languageEnglish
Article number084313
JournalJournal of Applied Physics
Volume109
Issue number8
DOIs
Publication statusPublished - 15 Apr 2011
Externally publishedYes

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ASJC Scopus subject areas

  • Physics and Astronomy(all)

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