### Abstract

A model of an isothermal bubble column slurry reactor for an arbitrary reaction network of R independent reactions and S reacting species has been developed. The model accounts for gas velocity variations due to a change in total number of moles during reaction, and for nonuniform catalyst distribution due to gravity settling. It is assumed that the gas phase is in plug flow and the batch liquid phase is unmixed, which is characteristic of pilot plant reactors with high aspect ratios. The minimum number of differential equations required for the complete description of the system is shown to be equal to the total number of independent reactions. A system of two series‐parallel reactions, representative of Fischer‐Tropsch synthesis, was used to study the effect of catalyst dispersion and model parameters on reactor performance. It was found that nonuniform catalyst distribution generally has a negative effect on conversion.

Original language | English |
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Pages (from-to) | 1197-1206 |

Number of pages | 10 |

Journal | AICHE Journal |

Volume | 33 |

Issue number | 7 |

DOIs | |

Publication status | Published - 1987 |

Externally published | Yes |

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### ASJC Scopus subject areas

- Biotechnology
- Environmental Engineering
- Chemical Engineering(all)

### Cite this

*AICHE Journal*,

*33*(7), 1197-1206. https://doi.org/10.1002/aic.690330714

**Modeling of bubble column slurry reactors for multiple reactions.** / Bukur, D. B.; Zimmerman, W. H.

Research output: Contribution to journal › Article

*AICHE Journal*, vol. 33, no. 7, pp. 1197-1206. https://doi.org/10.1002/aic.690330714

}

TY - JOUR

T1 - Modeling of bubble column slurry reactors for multiple reactions

AU - Bukur, D. B.

AU - Zimmerman, W. H.

PY - 1987

Y1 - 1987

N2 - A model of an isothermal bubble column slurry reactor for an arbitrary reaction network of R independent reactions and S reacting species has been developed. The model accounts for gas velocity variations due to a change in total number of moles during reaction, and for nonuniform catalyst distribution due to gravity settling. It is assumed that the gas phase is in plug flow and the batch liquid phase is unmixed, which is characteristic of pilot plant reactors with high aspect ratios. The minimum number of differential equations required for the complete description of the system is shown to be equal to the total number of independent reactions. A system of two series‐parallel reactions, representative of Fischer‐Tropsch synthesis, was used to study the effect of catalyst dispersion and model parameters on reactor performance. It was found that nonuniform catalyst distribution generally has a negative effect on conversion.

AB - A model of an isothermal bubble column slurry reactor for an arbitrary reaction network of R independent reactions and S reacting species has been developed. The model accounts for gas velocity variations due to a change in total number of moles during reaction, and for nonuniform catalyst distribution due to gravity settling. It is assumed that the gas phase is in plug flow and the batch liquid phase is unmixed, which is characteristic of pilot plant reactors with high aspect ratios. The minimum number of differential equations required for the complete description of the system is shown to be equal to the total number of independent reactions. A system of two series‐parallel reactions, representative of Fischer‐Tropsch synthesis, was used to study the effect of catalyst dispersion and model parameters on reactor performance. It was found that nonuniform catalyst distribution generally has a negative effect on conversion.

UR - http://www.scopus.com/inward/record.url?scp=0023386570&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=0023386570&partnerID=8YFLogxK

U2 - 10.1002/aic.690330714

DO - 10.1002/aic.690330714

M3 - Article

VL - 33

SP - 1197

EP - 1206

JO - AICHE Journal

JF - AICHE Journal

SN - 0001-1541

IS - 7

ER -