Abstract
The experimental atom probe tomography (APT) results from two different specimen orientations (top-down and sideways) of a high oxygen ion conducting Samaria-doped-ceria/Scandia-stabilized-zirconia multilayer thin film solid oxide fuel cell electrolyte was compared with level-set method based field evaporation simulations for the same specimen orientations. This experiment-simulation comparison explains the dynamic specimen shape evolution and ion trajectory aberrations that can induce density artifacts in final reconstruction, leading to inaccurate estimation of interfacial intermixing. This study highlights the importance of comparing experimental results with field evaporation simulations when using APT to study oxide heterostructure interfaces.
| Original language | English |
|---|---|
| Article number | 091601 |
| Journal | Applied Physics Letters |
| Volume | 107 |
| Issue number | 9 |
| DOIs | |
| Publication status | Published - 31 Aug 2015 |
Fingerprint
ASJC Scopus subject areas
- Physics and Astronomy (miscellaneous)
Cite this
Impact of dynamic specimen shape evolution on the atom probe tomography results of doped epitaxial oxide multilayers : Comparison of experiment and simulation. / Madaan, Nitesh; Bao, Jie; Nandasiri, Manjula; Xu, Zhijie; Thevuthasan, Suntharampillai; Devaraj, Arun.
In: Applied Physics Letters, Vol. 107, No. 9, 091601, 31.08.2015.Research output: Contribution to journal › Article
}
TY - JOUR
T1 - Impact of dynamic specimen shape evolution on the atom probe tomography results of doped epitaxial oxide multilayers
T2 - Comparison of experiment and simulation
AU - Madaan, Nitesh
AU - Bao, Jie
AU - Nandasiri, Manjula
AU - Xu, Zhijie
AU - Thevuthasan, Suntharampillai
AU - Devaraj, Arun
PY - 2015/8/31
Y1 - 2015/8/31
N2 - The experimental atom probe tomography (APT) results from two different specimen orientations (top-down and sideways) of a high oxygen ion conducting Samaria-doped-ceria/Scandia-stabilized-zirconia multilayer thin film solid oxide fuel cell electrolyte was compared with level-set method based field evaporation simulations for the same specimen orientations. This experiment-simulation comparison explains the dynamic specimen shape evolution and ion trajectory aberrations that can induce density artifacts in final reconstruction, leading to inaccurate estimation of interfacial intermixing. This study highlights the importance of comparing experimental results with field evaporation simulations when using APT to study oxide heterostructure interfaces.
AB - The experimental atom probe tomography (APT) results from two different specimen orientations (top-down and sideways) of a high oxygen ion conducting Samaria-doped-ceria/Scandia-stabilized-zirconia multilayer thin film solid oxide fuel cell electrolyte was compared with level-set method based field evaporation simulations for the same specimen orientations. This experiment-simulation comparison explains the dynamic specimen shape evolution and ion trajectory aberrations that can induce density artifacts in final reconstruction, leading to inaccurate estimation of interfacial intermixing. This study highlights the importance of comparing experimental results with field evaporation simulations when using APT to study oxide heterostructure interfaces.
UR - http://www.scopus.com/inward/record.url?scp=84940706608&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=84940706608&partnerID=8YFLogxK
U2 - 10.1063/1.4929705
DO - 10.1063/1.4929705
M3 - Article
AN - SCOPUS:84940706608
VL - 107
JO - Applied Physics Letters
JF - Applied Physics Letters
SN - 0003-6951
IS - 9
M1 - 091601
ER -